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https://support.microsoft.com/en-us/windows/about-sync-settings-on-windows-10-devices...

To find Sync settings, select the Start, then select Settings > Accounts > Sync your settings. To stop syncing your settings and remove them from the cloud, turn off synced settings on all the devices connected to your Microsoft account. Once this is done, you'll need to remove it from your account.

https://support.microsoft.com/en-us/microsoft-edge/change-and-customize-sync-settings...

Choose your sync settings in Microsoft Edge on your computer In the top corner of the browser window, select Settings and more, or use the keyboard shortcut Alt+F, and select Settings. Under Profiles > Your profile, select the profile you’d like to change the settings for, and select Sync.

https://docs.microsoft.com/answers/questions/478232/force-39sync-your-settings39-on...

To clarify this issue, please check if we could configure this setting -'Sync your settings' manually. Based on my experience, the settings are greyed out. And I also check this in an unenrolled device, it shows the same. If we couldn't configure this setting manually, I don't think we could force 'Sync your settings' via Intune.